SOLA
Online ISSN : 1349-6476
ISSN-L : 1349-6476
Article
Evaluation of Stratospheric Age of Air Estimated from Halocarbon Measurements of Air Samples Collected by a Balloon-Borne Cryogenic Air Sampler over Japan
Taku Umezawa, Satoshi Sugawara, Shoko Hikichi, Shinji Morimoto, Takuya Saito, Paul B. Krummel, Paul J. Fraser, Ray F. Weiss
著者情報
  • Taku Umezawa

    Earth System Division, National Institute for Environmental Studies

  • Satoshi Sugawara

    Faculty of Education, Miyagi University of Education

  • Shoko Hikichi

    Center for Atmospheric and Oceanic Studies, Tohoku University

  • Shinji Morimoto

    Center for Atmospheric and Oceanic Studies, Tohoku University

  • Takuya Saito

    Earth System Division, National Institute for Environmental Studies

  • Paul B. Krummel

    CSIRO Environment

  • Paul J. Fraser

    CSIRO Environment

  • Ray F. Weiss

    Scripps Institution of Oceanography, University of California San Diego

責任著者(Corresponding author)

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ジャーナル オープンアクセス

2025 年 21 巻 p. 237-243

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  • Published: 2025 Received: 2024年11月09日 Released on J-STAGE: 2025年06月09日 Accepted: 2025年04月23日 Advance online publication: 2025年05月11日 Revised: -
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To diagnose stratospheric transport, the mean age of air, the transit time of an air parcel from the troposphere to the stratosphere, has been estimated from measurements of trace gases, typically CO2 and SF6. Here we present a new set of halocarbon measurements on air samples collected at 15-35 km above Japan in 2020 using a balloon-borne cryogenic sampler. The mean ages of air were estimated based on a variety of trace gases combined with reference time series at the surface. The mean ages of air from HFC-23 and HFC-227ea showed general agreement to those derived from CO2 and SF6, which varied from < 2 yr below 20 km to almost constant values of ∼5 yr above ∼25 km altitude. In addition to conservation of the tracer in the stratosphere, measurement precision was found to be decisive to precisely estimate the mean age of air. We examined the age of air estimated from multiple tracers for future investigation towards improving assessment of the long-term trend in stratospheric circulation.

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© The Author(s) 2025. This is an open access article published by the Meteorological Society of Japan under a Creative Commons Attribution 4.0 International (CC BY 4.0) license.

This article is licensed under a Creative Commons [Attribution 4.0 International] license.
https://creativecommons.org/licenses/by/4.0/
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